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In the 2008-09 season she became topscorer of the Women Eredivisie with 14 goals. In the season 2009-10 she became topscorer again with 11 goals but had to share the honor with Chantal de Ridder (AZ).
On 6 August 2004 Smit debuted for the senior Netherlands women's national football team, playing the first half of a 2–0 friendly defeat to Japan in Zeist.
Smit also featured in the Netherlands' run to the semi-final of UEFA Women's Euro 2009.
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